In no particular order....

Television series
Full metal alchemist - I don't think I've ever cried as much as when I watched this O.o
Wolf's Rain - its the story that never ends ^^
Canaan - kick ass action scenes hands down, I will marry Alphard by any means necessary
Puella Madoka Magica - the story really confused me but it ended on a delightfully strange and sentimental note, along with great music and amazing art direction, Homura FTW
Ergo Proxy - such smooth animation...characters...this one definitely holds a place in my heart

Movies
Black rock shooter - I prefer these close combat fight scenes to shootouts, it's a must see if you enjoy beautiful fight scenes

1 - Gintama
2 - Baccano!
3 - Welcome to the NHK
4 - Durarara!!
5 - Shiki